Hydrogen Production by Homogeneous Partial Oxidation of Propane
Identifieur interne : 000951 ( Main/Exploration ); précédent : 000950; suivant : 000952Hydrogen Production by Homogeneous Partial Oxidation of Propane
Auteurs : Céline Hognon [France] ; Yves Simon [France] ; Paul-Marie Marquaire [France]Source :
- Energy & fuels [ 0887-0624 ] ; 2012.
Descripteurs français
- Pascal (Inist)
- Wicri :
- topic : Propane.
English descriptors
- KwdEn :
Abstract
A kinetic study of the partial oxidation of propane was performed in a jet stirred reactor. The main goal of this study was to establish a detailed homogeneous mechanism of this reaction and explore the capability to produce H2 and olefins. Various operating parameters are modified: temperature, residence time, and O2/C3H8 ratio. The mechanism was validated by comparing experimental and simulated results. A different behavior was observed depending on the temperature. At 600 °C, the mechanism contains both an oxidation and a pyrolytic path. The main products are H2, C2H4, CH4, CO, and O2. At 800 °C, the mechanism mostly contains a pyrolytic path. The main products are H2 and CO.
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Affiliations:
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Le document en format XML
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<series><title level="j" type="main">Energy & fuels</title>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Homogeneous reaction</term>
<term>Hydrogen production</term>
<term>Kinetics</term>
<term>Olefin</term>
<term>Partial oxidation</term>
<term>Propane</term>
<term>Reaction mechanism</term>
<term>Residence time</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Production hydrogène</term>
<term>Oxydation partielle</term>
<term>Propane</term>
<term>Cinétique</term>
<term>Réaction homogène</term>
<term>Mécanisme réaction</term>
<term>Oléfine</term>
<term>Temps séjour</term>
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<front><div type="abstract" xml:lang="en">A kinetic study of the partial oxidation of propane was performed in a jet stirred reactor. The main goal of this study was to establish a detailed homogeneous mechanism of this reaction and explore the capability to produce H<sub>2</sub>
and olefins. Various operating parameters are modified: temperature, residence time, and O<sub>2</sub>
/C<sub>3</sub>
H<sub>8</sub>
ratio. The mechanism was validated by comparing experimental and simulated results. A different behavior was observed depending on the temperature. At 600 °C, the mechanism contains both an oxidation and a pyrolytic path. The main products are H<sub>2</sub>
, C<sub>2</sub>
H<sub>4</sub>
, CH<sub>4</sub>
, CO, and O<sub>2</sub>
. At 800 °C, the mechanism mostly contains a pyrolytic path. The main products are H<sub>2</sub>
and CO.</div>
</front>
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<tree><country name="France"><region name="Grand Est"><name sortKey="Hognon, Celine" sort="Hognon, Celine" uniqKey="Hognon C" first="Céline" last="Hognon">Céline Hognon</name>
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<name sortKey="Marquaire, Paul Marie" sort="Marquaire, Paul Marie" uniqKey="Marquaire P" first="Paul-Marie" last="Marquaire">Paul-Marie Marquaire</name>
<name sortKey="Simon, Yves" sort="Simon, Yves" uniqKey="Simon Y" first="Yves" last="Simon">Yves Simon</name>
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